Regulated Li+ Solvation via Competitive Coordination Mechanism of Organic Cations for High Voltage and Fast Charging Lithium Metal Batteries
Jiangtao Yu,
Xinyu Ma,
Xiuyang Zou
et al.
Abstract:Li+ solvation exerted a decisive effect on electrolyte physicochemical properties. Suitable tuning for Li+ solvation enabled batteries to achieve unexpected performance. Here, we introduced inert organic cations to compete with Li+ for combining electrolyte molecules to modulate Li+ coordination in the electrolyte. The relevance between the number of cationic sites in organic cations and the competitive solvation ability was explored. The organic cations with multiple cationic sites attracted solvent molecules… Show more
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