2024
DOI: 10.1002/lpor.202401379
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Regulating Second‐Harmonic Generation in 2D Chiral Perovskites Through Achiral Organic Spacer Cation Alloying Strategy

Junzi Li,
Zhihang Guo,
Meiting Wang
et al.

Abstract: The inherent structural flexibility and chiroptical activity of 2D chiral perovskites make them promising for the nonlinear optical (NLO) application. A comprehensive understanding of the second‐harmonic generation (SHG) mechanism in 2D chiral perovskites is essential for developing NLO devices. However, the rational design of 2D chiral perovskite structures to regulate SHG properties remains challenging. Herein, to regulate SHG response, an achiral organic spacer cation alloying strategy is employed to constr… Show more

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