Regulation and synthesis of metal–organic frameworks through mixed-ligand strategy: A pathway to enhance adsorption of perfluoroalkyl acids

Sun, Yongxing; Quan, Kaijun; He, Jing; Chen, Jia; Li, Zuguang; Qiu, Hongdeng

doi:10.1016/j.cej.2024.153621

Chemical Engineering Journal

2024

DOI: 10.1016/j.cej.2024.153621

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Regulation and synthesis of metal–organic frameworks through mixed-ligand strategy: A pathway to enhance adsorption of perfluoroalkyl acids

Yongxing Sun,

Kaijun Quan,

Jing He

et al.

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Cited by 2 publications

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Trace Adsorptive Removal of PFAS from Water by Optimizing the UiO‐66 MOF Interface

Ilić,

Tan,

Mayr

et al. 2024

Advanced Materials

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The confluence of pervasiveness, bioaccumulation, and toxicity in freshwater contaminants presents an environmental threat second to none. Exemplifying this trifecta, per‐ and polyfluoroalkyl substances (PFAS) present an alarming hazard among the emerging contaminants. State‐of‐the‐art PFAS adsorbents used in drinking water treatment, namely, activated carbons and ion‐exchange resins, are handicapped by low adsorption capacity, competitive adsorption, and/or slow kinetics. To overcome these shortcomings, metal–organic frameworks (MOFs) with tailored pore size, surface, and pore chemistry are promising alternatives. Thanks to the compositional modularity of MOFs and polymer–MOF composites, herein we report on a series of water‐stable zirconium carboxylate MOFs and their low‐cost polymer‐grafted composites as C8–PFAS adsorbents with benchmark kinetics and “parts per billion” removal efficiencies. Bespoke insights into the structure–function relationships of PFAS adsorbents are obtained by leveraging interfacial design principles on solid sorbents, creating a synergy between the extrinsic particle surfaces and intrinsic molecular building blocks.

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Trace Adsorptive Removal of PFAS from Water by Optimizing the UiO‐66 MOF Interface

Ilić,

Tan,

Mayr

et al. 2024

Advanced Materials

View full text Add to dashboard Cite

show abstract

Thiol-yne click postsynthesis of imidazole-functionalized cyclodextrin microporous organic network: A remarkable adsorbent for sulfonamide antibiotics

Yue,

Wang,

Cui

et al. 2025

Separation and Purification Technology

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Regulation and synthesis of metal–organic frameworks through mixed-ligand strategy: A pathway to enhance adsorption of perfluoroalkyl acids

Cited by 2 publications

References 59 publications

Trace Adsorptive Removal of PFAS from Water by Optimizing the UiO‐66 MOF Interface

Trace Adsorptive Removal of PFAS from Water by Optimizing the UiO‐66 MOF Interface

Thiol-yne click postsynthesis of imidazole-functionalized cyclodextrin microporous organic network: A remarkable adsorbent for sulfonamide antibiotics

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