“…[7][8][9][10][11] We report here to the best of our knowledge, on the first studies of isotopic tracing of N, O, and H during thermal growth of oxynitride films in a RTP furnace in the synergistic gas sequences reported in Refs. 7-11, namely ͑i͒ growth of a SiO 2 film in O 2 , followed by nitridation in NH 3 , and then followed by reoxynitridation in N 2 O͑O 2 →NH 3 →N 2 O, samples 1-5 in Table I͒, [7][8][9] and ͑ii͒ growth of oxynitride films in N 2 O, followed by renitridation in NH 3 ͑N 2 O→NH 3 , samples 6-8͒. 10,11 Isotopically enriched gases were used for the RTP growth, namely, 99% 18 Table I, together with the total amounts of all isotopes present in the resulting oxynitride films as measured by nuclear reaction analyses ͑NRA͒.…”