Neuromorphic computing could enable
the potential to break the
inherent limitations of conventional von Neumann architectures, which
has led to widespread research interest in developing novel neuromorphic
memory devices, such as memristors and bioinspired artificial synaptic
devices. Covalent organic frameworks (COFs), as crystalline porous
polymers, have tailorable skeletons and pores, providing unique platforms
for the interplay with photons, excitons, electrons, holes, ions,
spins, and molecules. Such features encourage the rising research
interest in COF materials in neuromorphic electronics. To develop
high-performance COF-based neuromorphic memory devices, it is necessary
to comprehensively understand materials, devices, and applications.
Therefore, this Perspective focuses on discussing the use of COF materials
for neuromorphic memory devices in terms of molecular design, thin-film
processing, and neuromorphic applications. Finally, we provide an
outlook for future directions and potential applications of COF-based
neuromorphic electronics.