This report has been reproduced directly from the best available copy. Table 1 Table 2 Table 3 Table 4 Table 5 Table 6 Table 7 Table 8 Table 9 Table A1
ABSTRACTA Depleted Uranium Silicate Container Backfill System (DUSCOBS) is proposed that would use small, isotopicallydepleted uranium silicate glass beads as a backfill material inside storage, tramport, and repository waste packages containing spent nuclear fuel (SNF). The uranium silicate glass beads would fill all void space inside the package including the coolant channels inside SNF assemblies.Based on preliminary analysis, the following benefits have been identified. DUSCOBS improves repository waste package performance by three mechanisms. First, it reduces the radionuclide releases fiom SNF when water enters the waste package by creating a local uranium silicate saturated groundwater environment that suppresses (a) the dissolution andlor transformation of uranium dioxide fuel pellets and, hence, (b) the release of radionuclides incorporated into the SNF pellets. Second, the potential for long-term nuclear criticality is reduced by isotopic exchange of enriched uranium in SNF with the depleted uranium (DV) in the glass. Third, the backfill reduces radiation interactions bemeen SNF and the local environment (package and local geology) and thus reduces generation of hydrogen, acids, and other chemicals ;that degrade the waste package system. In addition, the DUSCOBS improves the integrity of the package by acting as a packing material and ensures criticality control for the package during SNF storage and transport. Finally, DUSCOBS provides a potential method to dispose of significant quantities of excess DU from uranium enrichment plants at potential economic savings. DUSCOBS is a new concept. Consequently, the concept has not been optimized or demonstrated in laboratow experiments.
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EXECUTIVE SUMMARY
INTRODUCTIONIt is proposed that small, depleted uranium silicate @US) glass beads be used as a backfill material inside storage, transport, and repository waste packages containing light-water reactor (LW) spent nuclear fuel (SNF). The use of DUS glass beads has the potential to improve repository performance, improve SNF transport and storage, dispose of excess depleted uranium (DU), and reduce system costs. A mechanical description of the Depleted Uranium Silicate Container Backfill System (DUSCOBS) is provided followed by descriptions of how DUSCOBS performs its functions. DUSCOBS is a new concept. This report is a first description of DUSCOBS, its potential advantages, and the associated uncertainties.For the study herein, DUSCOBS was applied to the proposed U.S. Department of Energy (DOE) multipurpose canister (MPC) system. The MPC is an inner container for SNF storage containers, transport casks, and geological disposal packages. DUSCOBS is applicable to (1) alternative MPC designs and (2) other SNF transport, storage, and repository systems.
MECHAMCAL DESCRIPTIONThe multipurpose canister (MPC) or waste package would first be loaded w...