2020
DOI: 10.5194/mr-2020-21
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Representation of population exchange at level anti-crossings

Abstract: Abstract. A theoretical framework is proposed to describe the spin dynamics driven by coherent spin mixing at Level Anti-Crossings (LACs). We briefly introduce the LAC concept and propose to describe the spin dynamics using a vector of populations of the diabatic eigenstates. In this description, each LAC gives rise to a pairwise redistribution of eigenstate populations, allowing one to construct the total evolution operator of the spin system. Additionally, we take into account that in the course of spin evol… Show more

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