2018
DOI: 10.1016/j.jnucmat.2018.05.043
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Research on chemical durability of iron phosphate glass wasteforms vitrifying SrF2 and CeF3

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Cited by 17 publications
(12 citation statements)
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“…Fluoride‐based nuclear wastes are challenging to immobilize in borosilicate glass, the most widely used class of wasteform material, due to both fluoride gas generation and the low solubility of fluoride in the glass matrix. The oxidation of fluoride waste into an oxide form followed by vitrification in borosilicate glass could be an option, but additional reprocessing may not be economically viable and will result in secondary waste generation 1,3 . Hence, it is vital to design and establish chemically and mechanically stable, durable wasteform alternatives to incorporate fluoride‐based radioactive wastes with reasonable waste loadings for safe disposal.…”
Section: Introductionmentioning
confidence: 99%
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“…Fluoride‐based nuclear wastes are challenging to immobilize in borosilicate glass, the most widely used class of wasteform material, due to both fluoride gas generation and the low solubility of fluoride in the glass matrix. The oxidation of fluoride waste into an oxide form followed by vitrification in borosilicate glass could be an option, but additional reprocessing may not be economically viable and will result in secondary waste generation 1,3 . Hence, it is vital to design and establish chemically and mechanically stable, durable wasteform alternatives to incorporate fluoride‐based radioactive wastes with reasonable waste loadings for safe disposal.…”
Section: Introductionmentioning
confidence: 99%
“…Several studies on incorporation of simulated fluoride waste from MSR were reported on phosphate glass, primarily due to lower melting temperature and relatively high solubility of halides 3 . Sodium aluminophosphate glass with waste loading 20 mol% (18.92 wt%) was reported by Sun et.al, 4,5 but crystallization occurs with a waste loading of 27.5 mol% (24.29 wt%).…”
Section: Introductionmentioning
confidence: 99%
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