2010
DOI: 10.1364/ol.35.003571
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Resonant optothermoacoustic detection: technique for measuring weak optical absorption by gases and micro-objects

Abstract: We report a laser spectroscopy technique for detecting optical absorption in gases and micro-objects via linked thermal effects and by using a sharp mechanical resonance in a quartz crystal. The performance of this technique is studied using near-IR diode lasers and two gases, pure CO(2) and C(2)H(2) diluted in nitrogen. A 7.3 × 10(-8) cm(-1)W/(Hz)(1/2) noise equivalent sensitivity to absorption in gases is demonstrated. Based on experimental results, it was estimated that 10(-8) fractional absorption of optic… Show more

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Cited by 23 publications
(25 citation statements)
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“…Other QEPAS spectrophone confi gurations, such as off-beam QEPAS, are also possible (Liu et al ., 2009(Liu et al ., , 2010. Furthermore, two novel modifi cations of the QEPAS sensor architecture based on interferometric photoacoustic spectroscopy (K ö hring et al ., 2011) and resonant optothermoacoustic detection (Kosterev and Doty, 2010 ) were reported recently.…”
Section: Conventional and Quartz-enhanced Photoacoustic Spectroscopymentioning
confidence: 94%
“…Other QEPAS spectrophone confi gurations, such as off-beam QEPAS, are also possible (Liu et al ., 2009(Liu et al ., , 2010. Furthermore, two novel modifi cations of the QEPAS sensor architecture based on interferometric photoacoustic spectroscopy (K ö hring et al ., 2011) and resonant optothermoacoustic detection (Kosterev and Doty, 2010 ) were reported recently.…”
Section: Conventional and Quartz-enhanced Photoacoustic Spectroscopymentioning
confidence: 94%
“…8 Radiation from a near-IR diode laser is coupled to a single mode fiber, and then focused between the prongs of the QTF with a waist size of ≈ 15μm. The position of the beam was controlled by moving the focusing optics with a computer controlled 3D translation stage (Newport ESP300 Motion Controller w/3D stage).…”
Section: Methodsmentioning
confidence: 99%
“…Recently it was shown that the same transducer that was used in QEPAS could be used as a mechanically resonant optothermal detector. 8 Resonant optothermoacoustic detection (ROTADE) occurs when the optically excited gas molecules impact the wall of the QTF and cause localized heating. The QTF deforms due to the localized heating and the piezo-electric quartz converts the deformation into an electrical signal.…”
Section: Introductionmentioning
confidence: 99%
“…The resulting temperature variations are detected indirectly via the pyroelectric effect and the result is thermal expansion in the tuning fork [12]. Clearly, this mechanism depends on the surrounding air pressure.…”
Section: Principlementioning
confidence: 99%