For
high-performance and high-lifetime flexible and wearable electronic
applications, a low-temperature posttreatment method is highly expected
to enhance the device performance and repair the defects induced by
the low-temperature fabrication process intrinsically. Particularly,
if the method can repair the traces induced by the multiple cycles
of bending or deforming, it would overcome current fatal obstacles
and provide a vital solution to the rapid development of flexible
electronics. In this work, we propose a method to apply low-temperature
supercritical CO2 fluid with a dehydration function to
improve or even restore the performance of flexible amorphous indium
gallium zinc oxide (a-IGZO) thin-film transistors (TFTs). After the
treatment, the a-IGZO TFT exhibits 3 times improvement drivability
up to 0.24 μA/μm, a smaller subthreshold swing of 0.18
V dec–1, a smaller V
th of 0.25 V, and a larger I
on/I
off ratio of 3.8 × 107. Additionally,
the posttreated a-IGZO TFTs possess relatively good uniformity and
reproducibility with an on-current standard deviation of 0.047 μA/μm,
and the performance of the a-IGZO TFT after the treatment remains
almost unchanged even after bending 2500 times at a bending radius
of 5 mm. These characteristics are attributed to the improved quality
of the channel and gate dielectric. It is worth noting that when this
is applied to a flexible TFT-driven organic light-emitting diode lighting
system, this treatment method can restore the performance of not only
the TFT but also the lighting system, even after the system has been
bent more than 600 times and has failed. To date, this is the first
time that the bending-track erasing function of the supercritical
fluid for flexible systems has been reported, which has the potential
to prolong the lifetime of flexible electronics.