Dielectric elastomer actuators (DEAs) are soft electromechanical devices that exhibit large energy densities and fast actuation rates. They are typically produced by planar methods and, thus, expand in-plane when actuated. Here, reported is a method for fabricating 3D interdigitated DEAs that exhibit in-plane contractile actuation modes. First, a conductive elastomer ink is created with the desired rheology needed for printing high-fidelity, interdigitated electrodes. Upon curing, the electrodes are then encapsulated in a self-healing dielectric matrix composed of a plasticized, chemically crosslinked polyurethane acrylate. 3D DEA devices are fabricated with tunable mechanical properties that exhibit breakdown fields of 25 V µm −1 and actuation strains of up to 9%. As exemplars, printed are prestrainfree rotational actuators and multi-voxel DEAs with orthogonal actuation directions in large-area, out-of-plane motifs.The ORCID identification number(s) for the author(s) of this article can be found under https://doi.org/10.1002/adfm.201907375.cycling and breakdown behavior [33][34][35] and the presence of a rigid frame limits the geometries that can be achieved. [24,36] Recent attention has been directed toward developing approaches that enable contractile displacements in prestrain-free DEAs, including manual and automated stacking of individual planar layers [37] or sequential deposition of active materials via inkjet printing [38] and spray coating. [39] The fabrication of contractile actuators with vertically oriented electrodes offers a more promising approach (Figure 1b). While arrays of vertical electrodes can be patterned lithographically, new masks must be generated for each device design. [40][41][42] By contrast, 3D printing enables the rapid design and fabrication of soft materials in nearly arbitrary geometries. [43][44][45][46][47] For example, direct ink writing (DIW), an extrusion-based 3D printing method, has been used to pattern soft functional materials, including sensors, [48] stretchable electronics, [49] liquid crystalline elastomers, [50] and soft robots. [51,52] While this method has recently been used to print DEAs, they do not exhibit an in-plane contractile response. [52][53][54] Here, we create 3D DEAs composed of interdigitated vertical electrodes that are printed, cured, and encapsulated in an insulating dielectric matrix (Figure 1c). These prestrain-free contractile DEAs can be produced in nearly arbitrary geometries. During their actuation, the stress generated is given by σ = ε 0 ε r (E) 2 , where ε 0 is the vacuum permittivity, ε r is the dielectric constant, and E is the electric field. For small strains, the actuation strain (s z ) is s z = σ/E Y = ε 0 ε r (E) 2 /E Y , where E Y is the Young's modulus. Their actuation performance is therefore maximized by increasing the breakdown field and dielectric constant, while simultaneously reducing the elastic modulus of the matrix. Since variations in the dielectric thickness can cause localization of the electric field that results in p...