2009
DOI: 10.1103/physreva.80.050302
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Robust control of individual nuclear spins in diamond

Abstract: Isolated nuclear spins offer a promising building block for quantum information processing systems, but their weak interactions often impede preparation, control, and detection. Hyperfine coupling to a proximal electronic spin can enhance each of these processes. Using the electronic spin of the nitrogen-vacancy center as an intermediary, we demonstrate robust initialization, single-qubit manipulation, and direct optical readout of 13C, 15N, and 14N nuclear spins in diamond. These results pave the way for nitr… Show more

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Cited by 144 publications
(189 citation statements)
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References 31 publications
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“…Therefore, a nonmonotonic behavior can be changed by polarizing the spin bath in diamond. [46][47][48] Here we adopted this strategy 46-49 by making use of a level anti-crossing in the excited state of the NV center to polarize the nuclear spins in diamond. By applying magnetic field along the axis of NV center, the tripe-mode spin bath was converted to a single mode system, as shown in Fig.…”
Section: Resultsmentioning
confidence: 99%
“…Therefore, a nonmonotonic behavior can be changed by polarizing the spin bath in diamond. [46][47][48] Here we adopted this strategy 46-49 by making use of a level anti-crossing in the excited state of the NV center to polarize the nuclear spins in diamond. By applying magnetic field along the axis of NV center, the tripe-mode spin bath was converted to a single mode system, as shown in Fig.…”
Section: Resultsmentioning
confidence: 99%
“…The NV electron spin is coupled to the nuclear spin of the NV's own nitrogen atom (I 0 = 1 for 14 N isotope, I 0 = 1/2 for 15 N isotope) via hyperfine interaction A 0 S z 0 I z 0 , where A 0 = −2π · 2.16 MHz for 14 N and A 0 = 2π · 3.03 MHz for 14 N. 67,68 The nuclear spin relaxation is slow, so that for a single experimental run the nuclear spin state is constant, but changes randomly between different experimental runs.…”
Section: Nv Center Coupled To the Dilute Spin Bathmentioning
confidence: 99%
“…Manipulation of such systems often utilizes a combination of microwave (MW) excitation to drive electronic spin transitions and radiofrequency (RF) excitation to control nuclear spins [2,3,7,8]. Experimental techniques typically rely on sequential RF and MW pulses [2,3], but a better understanding of simultaneous MW and RF excitation may enable greater parallelism in manipulating few-spin systems.…”
Section: Introductionmentioning
confidence: 99%