Role of Platinum Loading on the Characteristics at the PEM Fuel Cell Cathode

Derendyaev, M. A.; Koryakin, D. V.; Filalova, Emiliia; Yalmaev, A. B.; Galin, Monique; Герасимова, Е. В.; Antipov, A. E.; Левченко, А. В.; Dobrovolsky, Yu. A.

doi:10.1134/s1995078020060087

Cited by 5 publications

(1 citation statement)

References 48 publications

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“…Pt-based carbon-supported catalysts are commonly used at the PEMFC cathode [1,2]. Such electrocatalysts have high activity and sufficient stability under standard operating conditions of PEMFCs.…”

Section: Introductionmentioning

confidence: 99%

Carbon-Supported Pt-SnO2 Catalysts for Oxygen Reduction Reaction over a Wide Temperature Range: Rotating Disk Electrode Study

et al. 2021

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Pt/C and Pt/x-SnO2/C catalysts (where x is mass content of SnO2) were synthesized using a polyol method. Their kinetic properties towards oxygen reduction reaction were studied by a rotating disk electrode (RDE) technique in a temperature range from 1 to 50 °C. The SnO2 content of catalyst samples was 5 and 10 wt.%. A quick evaluation of the catalyst activity, electrochemical behavior and average number of transferred electrons were performed using the RDE technique. It has been shown that the use of x-SnO2 (through modification of the carbon support) in a binary system together with Pt does not reduce the catalyst activity in the temperature range of 1–30 °C. The temperature rising up to 50 °C resulted in composite catalyst activity reduction at about 30%.

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Section: Introductionmentioning

confidence: 99%

Carbon-Supported Pt-SnO2 Catalysts for Oxygen Reduction Reaction over a Wide Temperature Range: Rotating Disk Electrode Study

et al. 2021

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Key challenges for the development of the hydrogen industry in the Russian Federation

Баженов

Dobrovolsky

Maximov

et al. 2022

Sustainable Energy Technologies and Assessments

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Effects of Cooling System Boundary Conditions on the Performance of Proton Exchange Membrane Fuel Cell: A Comprehensive Analysis

Wang

Ren

2023

Journal of Electrochemical Energy Conversion and Storage

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We developed a three-dimensional multiphysics numerical model of a Proton Exchange Mem-brane Fuel Cell (PEMFC) with a cathode mesh structure to investigate how coolant flow rate and temperature impact its performance. After experimentally validating the model, we compared the performance of the cathode mesh structure PEMFC with that of the traditional straight flow PEMFC. The results indicate that the cathode mesh structure PEMFC has a lower pressure drop and a more index of uniform distribution (IUD), leading to enhanced performance, better temperature distribution, and improved water management of the PEMFC. The investigation of the cooling system's operating parameters revealed that the temperature of the cathode catalyst layer in the PEMFC is the highest, while the temperature of the bipolar plate is the lowest. Of the nine cases that we evaluated, Case 7, with a coolant inlet temperature and flow rate of 303.15 K and 0.07 m s−1, respectively, yielded the highest power density and the lowest average temperature. The IUD of the PEM in Case 5 was 0.608, suggesting that the temperature distribution of the PEM is more uniform when the coolant inlet temperature and flow rate are 323.15 K and 0.05 m s−1, respectively. We have demonstrated through calculations that there is a strong correlation between temperature difference and IUDs. These findings have significant implications for the optimization and application of PEMFCs.

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Role of Platinum Loading on the Characteristics at the PEM Fuel Cell Cathode

Cited by 5 publications

References 48 publications

Carbon-Supported Pt-SnO2 Catalysts for Oxygen Reduction Reaction over a Wide Temperature Range: Rotating Disk Electrode Study

Carbon-Supported Pt-SnO2 Catalysts for Oxygen Reduction Reaction over a Wide Temperature Range: Rotating Disk Electrode Study

Key challenges for the development of the hydrogen industry in the Russian Federation

Effects of Cooling System Boundary Conditions on the Performance of Proton Exchange Membrane Fuel Cell: A Comprehensive Analysis

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