2024
DOI: 10.1021/acs.langmuir.3c04036
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Role of Surface Chemistry in Pyrrole Autoxidation

Nikhila C. Paranamana,
Matthias J. Young

Abstract: Chemical compounds in liquid hydrocarbon fuels that contain fivemembered pyrrole (Py) rings readily react with oxygen from air and polymerize through a process known as autoxidation. Autoxidation degrades the quality of fuel and leads to the formation of unwanted gum deposits in fuel storage vessels and engine components. Recent work has found that the rate of formation of these gum deposits is affected by material surfaces exposed to the fuel, but the origins of these effects are not yet understood. In this w… Show more

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