Ru nanoparticles decorating ferrocene-based metal-organic framework for efficient and stable water-splitting electrocatalyst

Wang, Hong; Zhang, Yuzhen; Wu, Guanping; Guo, Li; Wang, Yanzhong

doi:10.1016/j.ijhydene.2024.03.283

International Journal of Hydrogen Energy

2024

DOI: 10.1016/j.ijhydene.2024.03.283

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Ru nanoparticles decorating ferrocene-based metal-organic framework for efficient and stable water-splitting electrocatalyst

Hong Wang,

Yuzhen Zhang,

Guanping Wu

et al.

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Cited by 5 publications

References 48 publications

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Ferrocene‐Based Nickel Metal–Organic Framework Nanosheets as Efficient, Long‐Cycle Cathode Catalyst for Li‐CO₂ Battery

Chen,

Li,

Liu

et al. 2024

Adv Funct Materials

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Li‐CO2 batteries, as a novel type of secondary battery, show great potential for energy conversion and storage. However, challenges such as large electrode polarization and poor cycling performance, stemming from difficulties in decomposing discharge products, limit their practical application. Here, Ferrocene‐based nickel metal–organic framework (Ni‐Fc) nanosheets structure to act as cathode catalysts, prepared via a one‐pot solvothermal reaction. X‐ray absorption fine structure (XAFS) analysis shows that Ni metal forms abundant catalytic active centers with O coordination of carboxylic acid groups in ferrocene units. The Ni‐Fc‐based battery demonstrates a high discharge capacity of 18636 mAh g−1 and exhibits a cycle life exceeding 2000 h at a current of 200 mA g−1. Density functional theory (DFT) calculations indicate that the stronger interaction of Ni‐Fc with discharge intermediates and enhanced Li adsorption accelerate battery reaction kinetics. This study introduces novel catalyst design concepts aimed at achieving high‐performance CO2 reduction and oxidation, thereby advancing Li‐CO2 batteries toward practical application.

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Ferrocene‐Based Nickel Metal–Organic Framework Nanosheets as Efficient, Long‐Cycle Cathode Catalyst for Li‐CO₂ Battery

Chen,

Li,

Liu

et al. 2024

Adv Funct Materials

View full text Add to dashboard Cite

show abstract

Electron-reservoir applications of ferrocenes and other late transition-metal sandwich complexes: Flow batteries, sensing, catalysis, and biomedicine

Wang,

Astruc

2025

Coordination Chemistry Reviews

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Borides and sulfide quantum dots co-enhanced the electrochemical property of metal organic framework/Ni3S2 composites for high-performance supercapacitors

Wu,

Cai,

Wang

et al. 2025

Fuel

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Ru nanoparticles decorating ferrocene-based metal-organic framework for efficient and stable water-splitting electrocatalyst

Cited by 5 publications

References 48 publications

Ferrocene‐Based Nickel Metal–Organic Framework Nanosheets as Efficient, Long‐Cycle Cathode Catalyst for Li‐CO₂ Battery

Ferrocene‐Based Nickel Metal–Organic Framework Nanosheets as Efficient, Long‐Cycle Cathode Catalyst for Li‐CO₂ Battery

Electron-reservoir applications of ferrocenes and other late transition-metal sandwich complexes: Flow batteries, sensing, catalysis, and biomedicine

Borides and sulfide quantum dots co-enhanced the electrochemical property of metal organic framework/Ni3S2 composites for high-performance supercapacitors

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Product

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Ru nanoparticles decorating ferrocene-based metal-organic framework for efficient and stable water-splitting electrocatalyst

Cited by 5 publications

References 48 publications

Ferrocene‐Based Nickel Metal–Organic Framework Nanosheets as Efficient, Long‐Cycle Cathode Catalyst for Li‐CO2 Battery

Ferrocene‐Based Nickel Metal–Organic Framework Nanosheets as Efficient, Long‐Cycle Cathode Catalyst for Li‐CO2 Battery

Electron-reservoir applications of ferrocenes and other late transition-metal sandwich complexes: Flow batteries, sensing, catalysis, and biomedicine

Borides and sulfide quantum dots co-enhanced the electrochemical property of metal organic framework/Ni3S2 composites for high-performance supercapacitors

Contact Info

Product

Resources

About

Ferrocene‐Based Nickel Metal–Organic Framework Nanosheets as Efficient, Long‐Cycle Cathode Catalyst for Li‐CO₂ Battery

Ferrocene‐Based Nickel Metal–Organic Framework Nanosheets as Efficient, Long‐Cycle Cathode Catalyst for Li‐CO₂ Battery