Ru, Pt and Co clusters in zeolite micropores; EXAFS/FTIR/TPD characterization and catalytic behaviors in methane homologation

Ichikawa, Masaru; Tanaka, Toshihiro; Pan, Wei; Ohtani, Takahiro; Ohnishi, Ryuichiro; Shido, Takafumi

doi:10.1016/s0167-2991(96)80319-3

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1997

1999

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“…Recently there is an increasing interest to activate methane under non-oxidative conditions and convert it to higher hydrocarbons and aromatic compounds as alternative feedstocks for the petrochemical industry. 1,2 Some supported Pt and Ru catalysts yield C 2 -C 5 hydrocarbons and even benzene in the low-temperature homologation of methane [3][4][5] but continuous catalytic reaction does not proceed. It has been previously reported that on Mo-supported ZSM-5 zeolite catalysts, a considerable amount of benzene was produced at 973 K in 60-70% selectivity in the gas-phase products at lower methane conversion while only benzene and toluene have been observed as the aromatic products.…”

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confidence: 99%