Rücktitelbild: Regulated Incorporation of Two Different Metal Ions into Programmed Sites in a Duplex by DNA Polymerase Catalyzed Primer Extension (Angew. Chem. 26/2014)

Funai, Tatsuya; Nakamura, Junko; Miyazaki, Yuki; Kiriu, Risa; Nakagawa, Osamu; Wada, Shun‐ichi; Ono, Akira; Urata, Hidehito

doi:10.1002/ange.201401152

Angewandte Chemie

2014

DOI: 10.1002/ange.201401152

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Rücktitelbild: Regulated Incorporation of Two Different Metal Ions into Programmed Sites in a Duplex by DNA Polymerase Catalyzed Primer Extension (Angew. Chem. 26/2014)

Tatsuya Funai

Junko Nakamura

Yuki Miyazaki

et al.

Abstract: HgII‐ und AgI‐Ionen lösen in Abwesenheit eines Watson‐Crick‐passenden Nucleotids spezifisch die durch DNA‐Polymerase katalysierte Primerverlängerung über die Bildung des T‐HgII‐T‐ und des erst entdeckten C‐AgI‐T‐Basenpaars aus. In der Zuschrift auf zeigen H. Urata et al., dass dank der strikten Basenerkennung dieser Metallionen der geregelte Einbau der beiden verschiedenen Metallionen an programmierte Stellen des DNA‐Duplex möglich ist.

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In situ Formed Co(TCNQ)₂ Metal‐Organic Framework Array as a High‐Efficiency Catalyst for Oxygen Evolution Reactions

Wei

Ren

et al. 2018

Chemistry A European J

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Energy conversion and storage systems such as water splitting devices and metal-air batteries need excellent and energy-efficiency oxygen evolution reaction (OER) catalysts. This work reports the in situ development of sawtooth-like Co(TCNQ) (TCNQ=tetracyanoquinodimethane) metal-organic framework array on Co foil (Co(TCNQ) /Co) by means of a solution immersion method at room temperature. As an oxygen-evolving catalyst, the resulting Co(TCNQ) /Co demonstrates superior OER activity with overpotential of 310 mV to drive a geometrical catalytic current density of 15 mA cm in 1.0 M KOH. Notably, it also shows good long-term electrochemical durability with its activity being retained for at least 20 h and achieves a high turnover frequency of 0.66 mol O s at overpotential of 380 mV.

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In situ Formed Co(TCNQ)₂ Metal‐Organic Framework Array as a High‐Efficiency Catalyst for Oxygen Evolution Reactions

Wei

Ren

et al. 2018

Chemistry A European J

View full text Add to dashboard Cite

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Synthesis of Cobalt Phosphide Nanoparticles Supported on Pristine Graphene by Dynamically Self‐Assembled Graphene Quantum Dots for Hydrogen Evolution

Wang

Yuan

et al. 2017

ChemSusChem

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A highly active, durable, and low-cost hydrogen evolution reaction (HER) catalyst is desirable for energy storage through water splitting but its fabrication presents great challenges. Herein, mediated by dynamically self-assembled graphene quantum dots (GQDs), small, uniform, high-density, and well-dispersed CoP nanoparticles were grown in situ on pristine graphene for the first time. This hybrid nanostructure was then employed as HER electrocatalyst, showing an onset potential of 7 mV, an overpotential of 91.3 mV to achieve 10 mA cm , a Tafel slope of 42.6 mV dec , and an exchange current density of 0.1225 mA cm , all of which compare favorably to those of most reported non-noble-metal catalysts. The developed catalyst also exhibits excellent durability with negligible current loss after 2000 cyclic voltammetry cycles (+0.01 to -0.17 V vs. RHE) or 34 h of chronoamperometric measurement at an overpotential of 91.3 mV. This work not only develops a new strategy for the fabrication of high-performance and inexpensive electrocatalysts for HER but also provides scientific insight into the mechanism of the dynamically self-assembled GQDsmediated synthesis process.

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Selective detection of N6-methyladenine in DNA via metal ion-mediated replication and rolling circle amplification

et al. 2017

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Rücktitelbild: Regulated Incorporation of Two Different Metal Ions into Programmed Sites in a Duplex by DNA Polymerase Catalyzed Primer Extension (Angew. Chem. 26/2014)

Cited by 3 publications

References 0 publications

In situ Formed Co(TCNQ)₂ Metal‐Organic Framework Array as a High‐Efficiency Catalyst for Oxygen Evolution Reactions

In situ Formed Co(TCNQ)₂ Metal‐Organic Framework Array as a High‐Efficiency Catalyst for Oxygen Evolution Reactions

Synthesis of Cobalt Phosphide Nanoparticles Supported on Pristine Graphene by Dynamically Self‐Assembled Graphene Quantum Dots for Hydrogen Evolution

Selective detection of N6-methyladenine in DNA via metal ion-mediated replication and rolling circle amplification

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Rücktitelbild: Regulated Incorporation of Two Different Metal Ions into Programmed Sites in a Duplex by DNA Polymerase Catalyzed Primer Extension (Angew. Chem. 26/2014)

Cited by 3 publications

References 0 publications

In situ Formed Co(TCNQ)2 Metal‐Organic Framework Array as a High‐Efficiency Catalyst for Oxygen Evolution Reactions

In situ Formed Co(TCNQ)2 Metal‐Organic Framework Array as a High‐Efficiency Catalyst for Oxygen Evolution Reactions

Synthesis of Cobalt Phosphide Nanoparticles Supported on Pristine Graphene by Dynamically Self‐Assembled Graphene Quantum Dots for Hydrogen Evolution

Selective detection of N6-methyladenine in DNA via metal ion-mediated replication and rolling circle amplification

Contact Info

Product

Resources

About

In situ Formed Co(TCNQ)₂ Metal‐Organic Framework Array as a High‐Efficiency Catalyst for Oxygen Evolution Reactions

In situ Formed Co(TCNQ)₂ Metal‐Organic Framework Array as a High‐Efficiency Catalyst for Oxygen Evolution Reactions