2024
DOI: 10.1002/ange.202419630
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Sabatier Optimal of Mn‐N4 Single Atom Catalysts for Selective Oxidative Desulfurization

Hanfeng Ye,
Wandong Xing,
Fei Zhao
et al.

Abstract: Understanding the relationship of competitive adsorption between reactants is the prerequisite for high activity and selectivity in heterogeneous catalysis, especially the difference between the adsorption energies (Eads) of two reactive intermediates in Langmuir‐Hinshelwood (L‐H) models. Using oxidative dehydrogenation of hydrogen sulfide (H2S‐ODH) as a probe, we develop various metal single atoms on nitrogen‐doped carbon (M‐NDC) catalysts for controlling Eads‐H2S, Eads‐O2 and investigating the difference in … Show more

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