2024
DOI: 10.1021/acsmacrolett.4c00347
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Salt-Screened Transition toward Bulk-Like Water Dynamics near Polymeric Zwitterions

Shawn D. Mengel,
Audra J. DeStefano,
Thomas Webber
et al.

Abstract: The superior antifouling performance of zwitterionic materials is commonly linked to their hydration structure, in which tight surface binding of water molecules inhibits solute adsorption. However, there is comparatively little direct experimental data on the hydration water structure and dynamics around zwitterionic moieties, including the longer-range behavior of the hydration shell that modulates the approach of solutes to the polymer surface. This work experimentally probes the dynamics of the diffusing h… Show more

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