LI, ANG. Aligned Carbon Nanotube Sheet Piezoresistive Strain Sensors. (Under the direction of Dr. Philip Bradford). With the application of advanced composites rapidly increasing into the aerospace and transportation industries, real time structural health monitoring (SHM) systems are attracting great attention in the composites research community. Carbon nanotubes (CNTs) have a unique set of properties that may be used for the production of a new generation strain/damage sensing materials. This research is going to introduce a novel CNT ensemble based strain sensor. The CNT sheet strain sensors were made with aligned CNT sheets and fiberglass/epoxy prepregs in a very convenient and efficient way. To evaluate the piezoresistive performance of the sensors, various types of mechanical tests were conducted with real-time electrical data acquisition. Specimens with orthogonal CNTs orientations were tested independently to investigate the influence of CNT orientation on piezoresistive behavior. The working mechanisms during mechanical straining were also discussed accordingly. Generally, the tested sensors were found to exhibit fairly good sensing stability, linearity, sensitivity and repeatability at a useful functional strain range, which is favorable for health monitoring of advanced composite material structures. It was also demonstrated that the CNT orientations have great effect on the sensitivity of sensors, leading to other promising applications such as directional strain/stress monitoring. Finally, a pre-straining process was intentionally applied, which enhanced the linearity and long-term dynamic stability of the piezoresistive sensing performance.