Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest

Abstract

Abstract. The Amazon rainforest routinely experiences intense and long-lived biomass burning events that result in smoke plumes that cover vast regions. The spatial and temporal extent of the plumes and the complex pathways through which they interact with the atmosphere have proved challenging to measure for purposes of gaining a representative understanding of smoke impacts on the Amazonian atmosphere. In this study, we use multiple collocated satellite sensors on board AQUA and TERRA platforms to study the underlying smoke–cloud–radiation interactions during the diurnal cycle. An 18-year time series for both morning and afternoon overpasses is constructed, providing collocated measurements of aerosol optical depth (AOD; column-integrated aerosol extinction), cloud properties, top-of-atmosphere radiative fluxes, precipitation, and column water vapour content from independent sources. The long-term time series reduces the impact of interannual variability and provides robust evidence that smoke significantly modifies the Amazonian atmosphere. Low loadings of smoke (AOD ≤ 0.4) enhance convective activity, cloudiness, and precipitation, but higher loadings (AOD > 0.4) strongly suppress afternoon convection and promote low-level cloud occurrence. Accumulated precipitation increases with convective activity but remains elevated under high smoke loadings, suggesting fewer but more intense convective cells. Contrasting morning and afternoon cloud responses to smoke are observed, in line with recent simulations. Observations of top-of-atmosphere radiative fluxes support the findings and show that the response of low-level cloud properties and cirrus coverage to smoke results in a pronounced and consistent increase in top-of-atmosphere outgoing radiation (cooling) of up to 50 W m−2 for an AOD perturbation of +1.0. The results demonstrate that smoke strongly modifies the atmosphere over the Amazon via widespread changes to the cloud field properties. Rapid adjustments work alongside instantaneous radiative effects to drive a stronger cooling effect from smoke than previously thought, whilst contrasting morning and afternoon responses of liquid and ice water paths highlight a potential method for constraining aerosol impacts on climate. Increased drought susceptibility, land use change, and deforestation will have important and widespread impacts on the region over the coming decades. Based on this analysis, we anticipate that further increases in anthropogenic fire activity will associated with an overall reduction in regional precipitation and a negative forcing (cooling) on the Earth's energy budget.

Assessment of NO2 uncertainty impact on aerosol optical depth retrievals at a global scale

“…The direct effect of aerosols is associated with the absorption and scattering of solar radiation (Hobbs, 1993) while the indirect effect involves the interaction of aerosols with clouds by acting as cloud condensation nuclei and potentially altering cloud properties, precipitation, surface fluxes and the energy budget of the atmosphere (Rosenfeld et al, 2014;Herbert and Stier, 2023). Apart from the impact on climate and radiative forcing, aerosols also have adverse effects on human health leading to respiratory, cardiovascular and neurological diseases, hypertension, diabetes and even cancer (Lelieveld et al, 2015;Molina et al, 2020).…”