have emerged as promising materials for fabricating soft actuators. [12][13][14] LCNs combine the anisotropy of the constituent liquid-crystal (LC) molecules and the elasticity of polymer networks, and are capable of stimuli-responsive shape change at the macroscopic scale. LCNs can be actuated by various stimuli such as light, [15] heat, [16] solvent, [17] and humidity. [18] Being a clean, remote, and precisely controllable stimulus, light is a particularly attractive energy source. [19] The light-triggered deformation of an LCN actuator is governed by the alignment distribution of the constituent liquid-crystal molecules within the polymer network, and developing methods for precise control over the director distribution in order to obtain desired photoactuation mode is an important topic of research. [14,[20][21][22] Photoalignment has proven to be a successful technique in patterning complex alignments into liquid-crystalline materials [23][24][25] and in devising on-demand actuations into LCNs. [21] The technique is based on illuminating a thin photoresponsive layer, a "command surface," [26] with linearly polarized light. Upon illumination, the photoalignment layer becomes anisotropic, thereby changing the boundary conditions experienced by the liquid-crystal molecules in the vicinity, and forcing them to align either perpendicular [27] or parallel [28] to the light polarization. Photopatterning of director orientation can be achieved by spatially modulating the light polarization, [27] or exposure through mask(s). [28,29] White and co-workers have used a laser setup to raster scan a focussed laser beam with controlled polarization across the sample, and thus achieved local control in the director distribution. [30][31][32] Also spatial light modulators and digital micromirror devices have been used for high-throughput patterning. [17,[33][34][35] These demonstrations require either prepatterned masks or relatively complex optical set-ups for programming the desired director distribution.Herein, we use a laser projector with a microelectromechanical system (MEMS)-based scanning mirror assembly (PICO, Sony) to program the liquid-crystal alignment within a monolithic LCN film. Photopatterning is achieved by projecting an arbitrary computer-generated image onto the photoalignment layer, using predefined light polarization. The projector is capable of addressing a minimum feature size of 50 µm over an area of 25 × 14 mm 2 . A series of complex photoactuators, such as defect buckling, coiling strip with gradient in pitch, four-arm gripper, and bidirectional bending in an octopod, are demonstrated by engineering different director orientations via photopatterning. The photoactuators are fabricated by polymerizing LC monomer mixtures inside LC cells that have been A versatile, laser-projector-based method is demonstrated for programming alignment patterns into monolithic films of liquid crystal polymer networks. Complex images can be photopatterned into the polymer films with sub-100 µm resolution, using relative...