Atmospheric aerosol affects local, regional, and global climate by directly absorbing and scattering the incoming and outgoing solar radiation [1], indirectly by altering the cloud microphysical properties [2], and semi-directly by reducing cloud coverage [3]. Aerosols also have an adverse impact on human health -particularly regarding respiratory and cardiovascular diseases [4]. Black carbon (BC) is a strongly light-absorbing component of the atmospheric aerosol, mainly PM 2.5 [5] formed during incomplete combustion of fossil fuels, biofuels, and biomass burning [6]. BC contributes to global warming [7][8] by possibly altering precipitation patterns [9] and melting glaciers due to snow albedo reduction [10]. Due to rapid urbanization and industrialization during the last decade, India and China are the largest BC emitters in the world, contributing 25 to 30% of global emissions of BC Pol. J. Environ. Stud. Vol. 26, No. 4 (2017), 1443-1451 , with 1.55 being the monthly average ratio for nighttime and daytime concentrations. Monthly average diurnal variation showed two distinct peaks, at morning with 39.84 µgm -3 (7:00-8:00 IST (Indian Standard Time)), and at night with 35.55 µgm -3 (00:00 -1:00 IST);and two distinct valleys, with lowest BC concentration (7.11 µgm , consistent with the nighttime average. A clear negative correlation between BC mass concentration and wind speed (r = -0.75), relative humidity (r = -0.30) and temperature (r = -0.19) was observed. The back-trajectory at surface level (50 m and 500 m) mostly originated from northeastern India, and for higher altitude (5,000 m), from Middle-Eastern and Arabian countries, except during the last week of December (Indian Ocean). The ratio and difference between BC mass measured at 370 nm and 880 nm showed biomass burning being the dominant cause at night.