We probe the structure and composition of the atmospheres of 5 hot Jupiter exoplanets using the Hubble Space Telescope Wide Field Camera 3 (WFC3) instrument. We use the G141 grism (1.1-1.7 µm) to study and CoRoT-1b in transit, TrES-3b in secondary eclipse, and WASP-4b in both. This wavelength region includes a predicted absorption feature from water at 1.4 µm, which we expect to be nondegenerate with the other molecules that are likely to be abundant for hydrocarbon-poor (e.g. solar composition) hot Jupiter atmospheres. We divide our wavelength regions into 10 bins. For each bin we produce a spectrophotometric light curve spanning the time of transit and/or eclipse. We correct these light curves for instrumental systematics without reference to an instrument model. For our transmission spectra, our mean 1 − σ precision per bin corresponds to variations of 2.1, 2.8, and 3.0 atmospheric scale heights for TrES-2b, TrES-4b, and CoRoT-1b, respectively. We find featureless spectra for these three planets. We are unable to extract a robust transmission spectrum for WASP-4b. For our dayside emission spectra, our mean 1 − σ precision per bin corresponds to a planet-to-star flux ratio of 1.5 × 10 −4 and 2.1 × 10 −4 for WASP-4b and TrES-3b, respectively. We combine these estimates with previous broadband measurements and conclude that for both planets isothermal atmospheres are disfavored. We find no signs of features due to water. We confirm 1 Harvard-Smithsonian Center for Astrophysics, Cambridge, MA 02138, USA