Selective photo-oxidative coupling of amines to form C–N bonds using post synthetic modification of MIL-68-NH2 with metal acetylacetonate

El-Shahat, Mahmoud; Wassel, Ahmed R.; Abdelhameed, Reda M.

doi:10.1039/d3nj02852f

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Cited by 11 publications

(1 citation statement)

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“…MOFs was used as heterogeneous catalysts, biological materials, luminescent materials, gas storage & separation substrate, transportable fuels, solar cells and electronic devices, and drug release and biosensing substrates, and adsorbent materials for water treatment. 1–11…”

Section: Introductionmentioning

confidence: 99%

Synthesis and applications of porphyrin-based MOFs in removal of pesticide from wastewater: molecular simulations and experimental studies

Ayman.FM,

Taha,

Farghali

et al. 2023

CrystEngComm

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Section: Introductionmentioning

confidence: 99%

Synthesis and applications of porphyrin-based MOFs in removal of pesticide from wastewater: molecular simulations and experimental studies

Ayman.FM,

Taha,

Farghali

et al. 2023

CrystEngComm

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Application of Ni‐Based MOFs Catalyst in Oxidative Coupling Reaction of Benzylamine

Nguyen,

Tran,

Van Huynh

et al. 2024

ChemistrySelect

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Nanoparticles made of porous coordination polymers, known as metal‐organic frameworks (MOFs), are becoming increasingly popular in nanomaterials research, especially in catalytic applications. With their intricate architectures, MOFs make it possible to incorporate metal nodes, encapsulate substrates, and use functional linkers, all of which contribute to synergistic engineering. A Ni‐based metal‐organic framework sample was prepared by the solvothermal method with NiCl2.6H2O as a precursor of Ni metal and terephthalic (H2BDC) acid as a linker. The as‐synthesized NiBDC was verified by X‐ray diffraction (XRD), Fourier‐transform infrared spectroscopy (FT‐IR), scanning electron microscopy (SEM), scanning electron microscopy with energy dispersive X‐ray spectroscopy (SEM‐EDX), transmission electron microscopy (TEM), and N2 adsorption/desorption isotherms. Based on these findings, we applied the as‐synthesized NiBDC to the oxidative coupling reaction of benzylamine. The results revealed that with NiBDC as a heterogeneous catalyst, the oxidative coupling reaction of benzylamine achieved a performance of 92%. Furthermore, the catalyst maintains good stability after four catalytic cycles, with an efficiency of approximately 82%.

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Recent development towards the novel applications and future prospects for cellulose-metal organic framework hybrid materials: a review

Qamar,

Aslam,

Fatima

et al. 2024

Environ Sci Pollut Res

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Selective photo-oxidative coupling of amines to form C–N bonds using post synthetic modification of MIL-68-NH2 with metal acetylacetonate

Abstract: Significant attention has been paid to the conversion of benzylamine into very valuable organic intermediates via selective photocatalytic oxidation using modified MOFs with acetylacetonate linker.

Cited by 11 publications

References 49 publications

Synthesis and applications of porphyrin-based MOFs in removal of pesticide from wastewater: molecular simulations and experimental studies

Synthesis and applications of porphyrin-based MOFs in removal of pesticide from wastewater: molecular simulations and experimental studies

Application of Ni‐Based MOFs Catalyst in Oxidative Coupling Reaction of Benzylamine

Recent development towards the novel applications and future prospects for cellulose-metal organic framework hybrid materials: a review

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