Self-catalytic induced interstitial C-doping of Pd nanoalloys for highly selective electrocatalytic dehydrogenation of formic acid

Li, Jun; Cai, Lu; Liang, Xiaosi; Huang, Shuke; Wang, Xiaosha; Kang, Yongshuai; Zhao, Yongjian; Zhang, Lei; Zhao, Chenyang

doi:10.1016/j.jechem.2023.01.026

Journal of Energy Chemistry

2023

DOI: 10.1016/j.jechem.2023.01.026

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Self-catalytic induced interstitial C-doping of Pd nanoalloys for highly selective electrocatalytic dehydrogenation of formic acid

Jun Li

Lu Cai

Xiaosi Liang

et al.

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Cited by 5 publications

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Efficient Palladium Catalysts: Application and Challenges of Electrocatalytic Hydrodechlorination Technology in Wastewater Treatment

Li,

Kong

2023

ChemCatChem

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This review summarizes the research progress of palladium (Pd) catalysts in electrocatalytic hydrodechlorination (ECH) for the removal of chlorinated organic pollutants (COPs). ECH technology is a new type of green water treatment technology without secondary pollution, which has excellent removal effect on COPs. Pd is widely used in the field of ECH due to its excellent catalytic properties. However, the easy deactivation and high price of Pd have limited the application of Pd catalysts in practical wastewater treatment. Researchers have improved the performance of Pd catalysts for ECH by improving the morphological structure (dispersion, particle size, crystalline surface) and electronic states (electron‐rich Pd, electron‐deficient Pd). It is also found that modulation of the adsorption abilities of Pd catalysts can greatly improve the catalytic activity. The factors affecting the stability of Pd catalysts are also investigated, and the future large‐scale mature application of ECH technology is envisioned. The ability to prepare single‐atom Pd catalysts in a relatively simple way is a future direction, which will achieve 100% atom utilization and thus significantly reduce the cost of Pd. This review details the frontier research on Pd catalysts in the field of ECH, which can provide some good strategies for related researchers.

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Efficient Palladium Catalysts: Application and Challenges of Electrocatalytic Hydrodechlorination Technology in Wastewater Treatment

Li,

Kong

2023

ChemCatChem

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Subsurface carbon modification of Ni-Ga for improved selectivity in acetylene hydrogenation reaction

Dong,

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et al. 2024

Chinese Chemical Letters

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d-d Orbital coupling induced by crystal-phase engineering assists acetonitrile electroreduction to ethylamine

Huang,

Chen,

et al. 2024

Journal of Energy Chemistry

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Self-catalytic induced interstitial C-doping of Pd nanoalloys for highly selective electrocatalytic dehydrogenation of formic acid

Cited by 5 publications

References 55 publications

Efficient Palladium Catalysts: Application and Challenges of Electrocatalytic Hydrodechlorination Technology in Wastewater Treatment

Efficient Palladium Catalysts: Application and Challenges of Electrocatalytic Hydrodechlorination Technology in Wastewater Treatment

Subsurface carbon modification of Ni-Ga for improved selectivity in acetylene hydrogenation reaction

d-d Orbital coupling induced by crystal-phase engineering assists acetonitrile electroreduction to ethylamine

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