2005
DOI: 10.13182/fst05-a1014
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Self-Radiolysis of Tritiated Water: Experimental Study and Simulation

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Cited by 19 publications
(9 citation statements)
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“…18,58 Throughout this study, we assumed that tritiated water could simply be described as a "dilute" solution of 3 HOH in light water, with concentrations of low volumic activity (typically, less than $1 Ci per mL) so that dose-rate effects could be ignored. 25,59…”
Section: Monte-carlo Track Chemistry Simulationsmentioning
confidence: 99%
“…18,58 Throughout this study, we assumed that tritiated water could simply be described as a "dilute" solution of 3 HOH in light water, with concentrations of low volumic activity (typically, less than $1 Ci per mL) so that dose-rate effects could be ignored. 25,59…”
Section: Monte-carlo Track Chemistry Simulationsmentioning
confidence: 99%
“…After assembling the experimental setup, the purge gas was aerated for 90 min to remove the dissolved air containing mainly N 2 that would result in nitric acid in tritiated water due to radiolysis, [12][13][14] and to equilibrate the [DO] in the electrolyte with purge gas containing 0$20% O 2 . The potential was kept at À0:7 V vs. AgjAgCl for 10 min as a cathodic treatment to remove the natural oxide layer, and thereafter remained an open circuit for 30 min.…”
Section: Methodsmentioning
confidence: 99%
“…The reaction of unlabeled water (H 2 O) with beta particles (produced from radiolysis of T 2 O) affords both stable molecular species (H 2 , H 2 O 2 , and O 2 ) and radicals 61–68 . The rates of evolution of H 2 and O 2 of a 1800 Ci/L T 2 O in water solution are 1.22 × 10 −5 (±0.07) mol L −1 s −1 and 7.44 × 10 −6 (±0.45) mol L −1 s −1 , respectively 69,70 …”
Section: Self‐radiolysis Of T2omentioning
confidence: 99%