2024
DOI: 10.1021/acs.inorgchem.4c00801
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Semiconductive Behavior and Photoconductivity of Uranyl Dithiophosphinate Single Crystal

Junren Wang,
Liangwei Yang,
Dingrui Yin
et al.

Abstract: Herein, we detail the synthesis, structure, and photoconductivity of the uranyl dithiophosphinate single crystal UO2[S2P(C6H5)2]2(CH3OH)·CH3OH (denoted as U-DPDPP). The formation of bonds between uranyl ions and sulfur-based ligands endows U-DPDPP with a distinct electronic absorption property with a broadband spectrum spanning from 250 to 550 nm, giving rise to a unique semiconductive property. Under X-ray illumination, U-DPDPP displays a distinctive photoconductivity response, with a charge carrier mobility … Show more

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