Significantly enhanced thermal and water stability of heterostructured CsPbBr3/Cs4PbBr6@PbS nanocrystals

Ye, Shuai; Huang, Mei-Feng; Han, Qinxin; Song, Jun; Qu, Junle

doi:10.1016/j.jallcom.2023.171442

Cited by 9 publications

(1 citation statement)

References 44 publications

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“…These desirable properties make them highly promising for applications in light-emitting diodes (LEDs) [8][9][10][11], solar cells [12][13][14], gas-sensing detection [15][16][17], photodetectors [18], and other fields [19][20][21]. However, the practical application of cesium lead halide perovskite quantum dots is hindered by their poor stability in light, water, oxygen, and heat [22][23][24][25]. This is primarily due to their ionic properties and low formation energy, which make them susceptible to ion migration and structural decomposition.…”

Section: Introductionmentioning

confidence: 99%

Multi-Functional Ethylene-vinyl Acetate Copolymer Flexible Composite Film Embedded with Indium Acetate-Passivated Perovskite Quantum Dots

Huang,

Gao,

Zhang

et al. 2023

Polymers

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In recent years, all-inorganic cesium lead halide perovskite quantum dots have emerged as promising candidates for various optoelectronic applications, including sensors, light-emitting diodes, and solar cells, owing to their exceptional photoelectric properties. However, their commercial utilization has been limited by stability issues. In this study, we addressed this challenge by passivating the surface defects of CsPbBr3 quantum dots using indium acetate, a metal–organic compound. The resulting CsPbBr3 quantum dots exhibited not only high photoluminescence intensity, but also a remarkably narrow half-peak width of 19 nm. Furthermore, by embedding the CsPbBr3 quantum dots in ethylene-vinyl acetate, we achieved stretchability and significantly enhanced stability while preserving the original luminous intensity. The resulting composite film demonstrated the potential to improve the power conversion efficiency of crystalline silicon solar cells and enabled the creation of excellent white light-emitting diodes with coordinates of (0.33, 0.31). This co-passivation strategy, involving surface passivation and polymer packaging, provides a new idea for the practical application of CsPbBr3 quantum dots.

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