Visible light communication (VLC) has attracted widespread attention for wireless communications. The popularity of GaN-based light-emitting diodes (LEDs) has also laid a solid foundation for the application of VLC. As the light source of VLC, LED's modulation bandwidth directly determines the speed of communication. Herein, reviewing progress on modulation bandwidth improvement schemes of GaN LEDs transmitter is reviewed, covering aspects from epitaxial to devices. Epitaxial approaches include c-polar facet epitaxial optimization, non/semipolar facet epitaxial growth, and chip scheme such as micro-LEDs, nano-LEDs, resonant cavity-LEDs (RC-LEDs), plasmon, and metacavity LEDs. In terms of white LEDs, approaches to tackle the slow Stokes transfer and long carrier life for conventional phosphors including new color-conversion materials (CCMs) and new energy transfer routes are reviewed. This review promotes the development of GaN-based LEDs as the transmitter for high-speed VLC.