Background: Rotational bands have been measured around 250 Fm associated with strong deformed-shell closures. The K π = 2 − excited band emerges systematically in N = 150 isotones raging from plutonium to nobelium with even-Z numbers, and a sharp drop in energies was observed in californium.Purpose: I attempt to uncover the microscopic mechanism for the appearance of such a low-energy 2 − state in 248 Cf. Furthermore, I investigate the possible occurrence of the low-energy K π = 2 + state, the γ vibration, to elucidate the mechanism that prefers the simultaneous breaking of the reflection and axial symmetry to the breaking of the axial symmetry alone in this mass region.Method: I employ a nuclear energy-density functional (EDF) method: the Skyrme-Kohn-Sham-Bogoliubov and the quasiparticle random-phase approximation are used to describe the ground state and the transition to excited states.
Results:The Skyrme-type SkM* and SLy4 functionals reproduce the fall in energy but not the absolute value of the K π = 2 − state at Z = 98 where the proton two-quasiparticle excitation [633]7/2 ⊗ [521]3/2 plays a decisive role for the peculiar isotonic dependence. I find interweaving roles by the pairing correlation of protons and the deformed-shell closure at Z = 98. The SkM* model predicts the K π = 2 − state appears lower in energy in 246 Cf than in 248 Cf as the Fermi level of neutrons is located in between the [622]5/2 and the [734]9/2 orbitals. Except for 250 Fm in the SkM* calculation, the K π = 2 + state is predicted to appear higher in energy than the K π = 2 − state because the quasiproton [521]1/2 orbital is located above the [633]7/2 orbital.
Conclusions:A systematic study of low-lying collective states in heavy actinide nuclei provides a rigorous testing ground for microscopic nuclear models. The present paper shows a need for improvements in the EDFs to describe pairing correlations and shell structures in heavy nuclei, that are indispensable in predicting the heaviest nuclei.