To develop a flexible display, smartphones with edge screens with curved displays on both sides of the main screen have been used widely. Considering that small differences in the form of smartphones, such as length, width, and thickness, could affect user experience, the effects of the curvature of the edge screen should be identified. This study aimed to investigate the effects of the curvature of edge screens on subjective feelings of smartphone users and to find out the optimal curvature. In the experiment, four nonfunctional samples with different radii of curvature (4R/6R/8R/10R) were used as samples, and participants evaluated the five subjective feelings: grip/control comfort, front/side visibility, and stability of the samples with four usage patterns. Our results revealed that 8R is the optimal curvature for the edge screen based on subjective feelings in smartphone usage. Moreover, the effect of the curvature of the edge screen on grip comfort and control comfort varied according to the usage patterns. The results of this study can be applied to design of the curvature of edge screens in smartphones and it is expected that it will contribute to improvement of users’ satisfaction.