The fabrication of surface nanoscale axial photonics (SNAP) microresonators, utilizing the approach of electric arc discharge (EAD), is accomplished, achieving a precision at the angstrom level. This paper thoroughly investigates the effects that discharge intensity and discharge duration have on SNAP microresonators, respectively, through the manipulation of relevant discharge parameters. The results indicate that, within a specified range of discharge intensity, a linear relationship is observed between the effective radius variation (ERV) and the discharge intensity, characterized by a slope of 0.325 nm/intensity unit. As the discharge duration is extended, the ERV gradually increases, eventually reaching a saturation value, which is inherently determined by the discharge intensity. Additionally, as the discharge intensity (or time) continues to increase, a “convex–concave–convex” shape is observed on the fiber, providing a method for fabricating bat microresonators. These discoveries derived from our study contribute toward providing a strong foundation for the progressive enhancement and refinement of EAD-based SNAP fabrication techniques.