SnO2@MoS2 heterostructures grown on nickel foam as highly efficient bifunctional electrocatalyst for overall water splitting in alkaline media

He, Wurigamula; Wang, Lili; Zhang, Helin; Gao, Shuang; Yu, Wensheng; Yin, Duanduan; Dong, Xiangting

doi:10.1016/j.jallcom.2022.168678

Cited by 15 publications

(3 citation statements)

References 46 publications

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“…[ 61 ] Compared to SnSe, the Se 3 d peaks are negatively shifted in SnSe/SnTe, suggesting that extra charges in Se imply an increased capability to adsorb H* and OH*intermediates. [ 62 ] Figure 2d exhibits the deconvoluted XPS spectra of Te 3 d , which depict the peaks at binding energies of 582.7 and 572.3 eV corresponding to Te 3 d 3/2 and Te 3 d 5/2 . [ 63 ] The peak at a binding energy of 575.33 eV corresponds to the partial oxidation of Te on the surface.…”

Section: Resultsmentioning

confidence: 99%

Harnessing Wind Energy for Ultraefficient Green Hydrogen Production with Tin Selenide/Tin Telluride Heterostructures

Sajeev,

Perumalsamy,

Elumalai

et al. 2024

Small Science

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Industrialization of green hydrogen production through electrolyzers is hindered by cost‐effective electrocatalysts and sluggish oxygen evolution reaction (OER). Herein, a facile one‐step hydrothermal technique for the in situ growth of non‐noble tin chalcogenides and their heterostructures on nickel foam (NF) as trifunctional electrocatalysts for hydrogen evolution reaction (HER), OER, and methanol oxidation reaction (MOR) is detailed. Among them, the heterostructured SnSe/SnTe/NF outperforms all others and recently reported catalysts, boasting an impressively low potential of −0.077, 1.51, and 1.33 V versus reversible hydrogen electrode to achieve 10 mA cm−2 for HER, OER, and MOR. Owing to the rod‐like morphology with hetero‐phases for enhancing the performance. Furthermore, a hybrid MOR‐mediated water electrolyzer requiring only 1.49 V to achieve 10 mA cm−2 with value‐added formate is introduced and traditional water electrolyzer is outperformed. Additionally, a zero‐gap commercial anion‐exchange membrane water electrolyzer (AEMWE) with bifunctional SnSe/SnTe/NF electrodes is tested, successfully achieving an industrially required 1 A cm−2 at a low potential of 1.93 V at 70 °C. Moreover, AEMWE using a windmill is powered and H2 and O2 production with wind speed is measured. Overall, this work paves the development of unexplored tin chalcogenide heterostructure as a potent candidate for cost‐effective, energy‐efficient, and carbon‐neutral hydrogen production.

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Section: Resultsmentioning

confidence: 99%

Harnessing Wind Energy for Ultraefficient Green Hydrogen Production with Tin Selenide/Tin Telluride Heterostructures

Sajeev,

Perumalsamy,

Elumalai

et al. 2024

Small Science

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“…The bi-functional electrode, which possessed these distinct characteristics, demonstrated remarkable performance in alkaline water electrolysis. It accomplished 10 mA cm −2 at a cell voltage of 1.57 V and retained 98.3% of its initial current after 300 h of continuous testing, exhibiting exceptional long-term electrochemical stability [ 253 ]. The unique 3D structure of MoS 2 nanosheets anchored on Ni 9 S 8 nanorods has shown promising results in the field of water splitting.…”

Section: Energy Applicationsmentioning

confidence: 99%

Recent Advances in Molybdenum Disulfide and Its Nanocomposites for Energy Applications: Challenges and Development

et al. 2023

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Energy storage and conversion are critical components of modern energy systems, enabling the integration of renewable energy sources and the optimization of energy use. These technologies play a key role in reducing greenhouse gas emissions and promoting sustainable development. Supercapacitors play a vital role in the development of energy storage systems due to their high power density, long life cycles, high stability, low manufacturing cost, fast charging-discharging capability and eco-friendly. Molybdenum disulfide (MoS2) has emerged as a promising material for supercapacitor electrodes due to its high surface area, excellent electrical conductivity, and good stability. Its unique layered structure also allows for efficient ion transport and storage, making it a potential candidate for high-performance energy storage devices. Additionally, research efforts have focused on improving synthesis methods and developing novel device architectures to enhance the performance of MoS2-based devices. This review article on MoS2 and MoS2-based nanocomposites provides a comprehensive overview of the recent advancements in the synthesis, properties, and applications of MoS2 and its nanocomposites in the field of supercapacitors. This article also highlights the challenges and future directions in this rapidly growing field.

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“…12 The fusion of distinct quantum materials to create efficient heterostructures is drawing attention in the generation of maximum amounts of H 2 from photocatalytic watersplitting reactions. 13 Recently, different heterostructures have been introduced for water splitting, e.g., GaTe/ZnI 2 , 14 PG/GeP 2 and PG/SiP 2 , 15 ZnO/ZnS, 16 BiVO 4 /Zn 3 V 2 O 8 , 17 NiS/NiS 2 , 18 2Dporous Co-Mo nitrides, 19 BiVO 4 /CoFe MOF, 20 SnO 2 @MoS 2 , 21 C 2 N/ZnSe, 22 Ru@RuO 2 , 23 covalent triazine framework, 24 CdS/ quantum dots, 25,26 MXene supported catalysts, 27 transition metal chalcogenides, 28 nanosphere heterostructures, 29 etc. Despite some benefits, there have been reports of several drawbacks associated with them, such as wide band gap, inadequate stability, toxicity and high price.…”

Section: Introductionmentioning

confidence: 99%

Promoting water-splitting reaction on TiO₂/gCN with Pd/SrO cocatalysts: H₂ evolution in the absence of a sacrificial reagent

Rafiq,

Sahar,

Abid

et al. 2024

Energy Adv.

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SnO2@MoS2 heterostructures grown on nickel foam as highly efficient bifunctional electrocatalyst for overall water splitting in alkaline media

Cited by 15 publications

References 46 publications

Harnessing Wind Energy for Ultraefficient Green Hydrogen Production with Tin Selenide/Tin Telluride Heterostructures

Harnessing Wind Energy for Ultraefficient Green Hydrogen Production with Tin Selenide/Tin Telluride Heterostructures

Recent Advances in Molybdenum Disulfide and Its Nanocomposites for Energy Applications: Challenges and Development

Promoting water-splitting reaction on TiO₂/gCN with Pd/SrO cocatalysts: H₂ evolution in the absence of a sacrificial reagent

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SnO2@MoS2 heterostructures grown on nickel foam as highly efficient bifunctional electrocatalyst for overall water splitting in alkaline media

Cited by 15 publications

References 46 publications

Harnessing Wind Energy for Ultraefficient Green Hydrogen Production with Tin Selenide/Tin Telluride Heterostructures

Harnessing Wind Energy for Ultraefficient Green Hydrogen Production with Tin Selenide/Tin Telluride Heterostructures

Recent Advances in Molybdenum Disulfide and Its Nanocomposites for Energy Applications: Challenges and Development

Promoting water-splitting reaction on TiO2/gCN with Pd/SrO cocatalysts: H2 evolution in the absence of a sacrificial reagent

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Promoting water-splitting reaction on TiO₂/gCN with Pd/SrO cocatalysts: H₂ evolution in the absence of a sacrificial reagent