Solar steam generation (SSG) is an effective way to mitigate
the
freshwater crisis. However, challenges still remain in scalable preparation,
cost-effectiveness, and expanding the scope of practical applications
for photothermal materials. Herein, a biomass-based solar steam generator
(named OR-INP) with salt-resistant, oil-repellent, and anti-fouling
performances is fabricated by grafting poly(ionic liquid)s onto celluloses
from waste newspapers and then conducting oil-repellent modification.
Benefiting from the broad solar absorption in the wet state (ca. 92%), low thermal conductivity (0.1108 W m–1 K–1), and strong hydrophilic and oleophobic properties,
the solar evaporation efficiency is as high as 93.25% for pure water,
84.96% for 20 wt % NaCl, and 78.46% for 5 wt % oily wastewater, under
1 sun irradiation. Moreover, the aerogel still has excellent purification
effects on solutions which contain organic dyes, heavy metal ions,
or bacteria. Therefore, combining the merits of salt resistance, oil
repellency, and wastewater treatment, this work develops the prospect
of employing waste biomass resource-based photothermal materials and
expands the practical application range of biomass-based evaporators.