South Asia is experiencing a levelling-off trend in solar radiation and even a transition from dimming to brightening. Any change in incident solar radiation, which is the only significant energy source of the global ecosystem, profoundly affects our habitats. Here, we use multiple observations of the A-Train constellation to evaluate the impacts of three-dimensional (3D) aerosol, cloud, and water vapor variations on the changes in surface solar radiation during the monsoon season (June-September) in South Asia from 2006 to 2015. Results show that surface shortwave radiation (SSR) has possibly increased by 16.2 W m −2 during this period. However, an increase in aerosol loading is inconsistent with the SSR variations. Instead, clouds are generally reduced and thinned by approximately 8.8% and 280 m, respectively, with a decrease in both cloud water path (by 34.7 g m −2 ) and particle number concentration under cloudy conditions. Consequently, the shortwave cloud radiative effect decreases by approximately 45.5 W m −2 at the surface. Moreover, precipitable water in clear-sky conditions decreases by 2.8 mm (mainly below 2 km), and related solar brightening increases by 2.5 W m −2 . Overall, the decreases in 3D water vapor and clouds distinctly result in increased absorption of SSR and subsequent surface brightening.