“…However, classical nucleation theory has not been completely successful at explaining atmospheric nucleation events (Weber et al, 1997;Clarke et al, 1998a;Weber et al, 1999;Weber et al, 2001a). Alternative pathways for sulfate aerosol formation have been suggested, including neutral ternary nucleation of water, sulfuric acid, and ammonia (Coffman and Hegg, 1995;Marti et al, 1997;Korhonen et al, 1999), and charged (ion-induced) nucleation of water and sulfuric acid (Dickinson, 1975;Raes andJanssens, 1985, 1993;Yu and Turco, 2000). Ions are likely aerosol precursors because they greatly stabilize small clusters with respect to evaporation.…”