In this era of environmental protection and performance,
the development
of organic photodetectors is booming. The hydrogel material is beginning
to attract attention because of its characteristics such as plasticity
and ecofriendliness. However, it is still a challenge to achieve a
high-speed response in biophotodetectors. Herein, the development
of an organic one-dimensional nanostructured photodetector is proposed
through rotary-jet injection of gelatin fibers incorporated with silver
nanoparticles (Ag NPs). The variation in the photoelectric properties
of thin-film, fibrous structures with different diameters of approximately
40 μm and 400 nm has been investigated. In particular, the gelatin–Ag
NPs fiber photoreceptor with a diameter of about 400 nm improved the
light-to-dark current ratio by up to 28000% higher than the film structure,
with rise and decay times of only 0.23 and 0.56 s. In addition, the
nanostructure effectively boosts the photocurrent and suppresses the
dark current because of its confining domains. The Ag NPs within the
gelatin nanofibers produce localized surface plasmon resonance in
the UV-illumination environment, enhancing the light absorption of
the photosensitive layer, which contributes directly to the increase
in the rate of excitons. The novel structure of the hybridized gelatin
nanofibers incorporating silver nitrate has offered the promising
potential for organic photodetectors.