A novel adsorbent, magnetic nanoparticle (-Fe 2 O 3 )-coated zeolite (MNCZ), was prepared for the removal of arsenic (As) ions from aqueous solution. The influence of different sorption parameters, that is, contact time, acidic reaction (pH) and initial arsenic concentration were studied using batch equilibrium techniques. The results obtained showed that the MNCZ was effective for the removal of As from aqueous solution, and the percentage removal of As could reach over 95.6% at a pH value of 2.5 within 15 min. Moreover, the removal of As depended on the initial concentration of As. For the regeneration of MNCZ material, 0.1 M NaOH was suitable for the desorption of As (70% after 15 min), and the regenerated material showed an adsorption capacity of 93.95% within five cycles. We concluded that MNCZ presents a reusable adsorbent for a fast, convenient and highly efficient removal of As from aqueous solution.