The performance of a radiometric unmanned aircraft system (UAS) composed of a directional gamma spectrometer, the Advanced Radiation Detector for Unmanned Aircraft System Operations (ARDUO), and a medium-lift helicopter airframe was demonstrated. The ARDUO's properties of the full-width half maximum energy resolution, linearity, gain stability, intrinsic photopeak efficiency, sheet source sensitivity and directional response were characterized in laboratory experiments. Smallscale trials were conducted over a single point source and two point sources of 137 Cs at a 27 m separation. The single point source strength was measured at iii Statement of Contribution v Table of Contents vii List of Tables x List of Figures xi List of Acronyms xiv List of Symbols xvii List of Acronyms Acronym Meaning 40 Ar Argon-40 ARDUO Advanced Radiation Detector for Unmanned Aircraft System Operations 133 Ba Barium-133 Bi Bismuth-214 Bq, kBq, MBq, GBq Becquerel, disintegrations per second, kilo-becquerel, mega-becquerel, giga-becquerel Ci Curie 60 Co Co-60 cps Counts per second 137 Cs Cesium-137 CsI, CsI(Tl) Cesium iodide, thallium-doped cesium iodide CZT Cadmium zinc telluride EDT Eastern day time EKF Extended Kalman Filter xiv Acronym Meaning 152 Eu Europium-152 eV, keV, MeV Electron volt, kilo-electron volt, mega-electron volt FWHM Full-width half maximum g, kg Gram, kilogram GCS Ground Control Station GHz Gigahertz GNSS Global Navigation Satellite System 140 La Lanthanum-140 m, km, cm Metre, kilometre, centimetre MDT Mountain day time xv Acronym Meaning min Minute 54 Mn Magnesium-54 NaI, NaI(Tl) Sodium iodide, thallium-doped sodium iodide NRCan Natural Resources Canada RSI Radiation Solutions Inc. [5] RTL Return to Launch s, µs Second, microsecond