“…Such techniques have successfully been applied to line spectral data, and the topic has attracted notable attention in the recent literature (see, e.g., [5][6][7][8][9][10][11]). Although these algorithms appear quite different from each other, they share the property that the considered dictionary grid should be selected sufficiently fine to allow for a sparse signal representation (see also [12,13]), which, if extended to also consider damped modes, necessitates a large dictionary matrix containing elements with a sufficiently fine grid over the range of both the potential frequencies and damping candidates (see, e.g., [2,14,15]); this will be particularly noticeable if treating large data sets, or data sets with multiple measurement dimensions, such as in NMR measurements. In order to mitigate this problem, we here propose a novel dictionary learning approach wherein we iteratively decompose the signal with a fixed small dictionary, adaptively learning the dictionary elements best suited to enhance sparsity.…”