We report the development of a sputter erosion monitoring system to study Hall thruster lifetime and contamination. The laser-based sensor uses the continuous-wave cavity ring-down spectroscopy technique and allows for in situ measurements in near-real time. The continuous-wave cavity ring-down spectroscopy technique diagnostic allows direct probing of sputter products in their ground state, thereby providing a reliable quantitative measure of their overall number density. Combining the number density of sputtered particles with their velocity allows determination of the flux of sputtered particles and erosion rate. We perform proof of principle experiments, in which sputtered manganese atoms from the acceleration channel of an anode layer-type Hall thruster are measured. The measurement strategy is to detect the manganese atoms via an absorption line from the ground state at a wavelength of 403.076 nm (air). The measured path-integrated number density of sputtered manganese atoms is 1:7 0:3 10 13 m 2 for an argon anode mass flow rate of 2:08 mg=s and a discharge voltage of 250 V. A finite element sputter model is used to compare the cavity ring-down spectroscopy results against validating mass loss measurements and shows good agreement. Nomenclature A ki = Einstein A coefficient, 1=s Abs = absorbance c = speed of light, 2:998 10 8 m=s E b = binding energy, J E i = energy of state i, J E k = energy of state k, J g i = degeneracy of state i g k = degeneracy of state k k = absorption coefficient, m 1 l = length of the ring-down cavity, m l abs = path length of absorbing species, m N i = lower-state concentration, m 3 R = mirror reflectivity St; = ring-down signal as a function of time and laser frequency S 0 = initial ring-down signal x = position along the optical axis, m = laser frequency, Hz ki = resonant frequency of transition, Hz = ring-down time, s 0 = empty cavity ring-down time, s