The Gaussian transition in the spin-1 Heisenberg chain with single-ion anisotropy is extremely difficult to treat, both analytically and numerically. We introduce an improved density-matrix renormalization group procedure with strict error control, which we use to access very large systems. By considering the bulk entropy, we determine the Gaussian transition point to four-digit accuracy, D c /J = 0.968 45(8), resolving a long-standing debate in quantum magnetism. With this value, we obtain high-precision data for the critical behavior of quantities, including the ground-state energy, gap, and transverse string-order parameter, and for the critical exponent ν = 1.472(2). Applying our improved technique at J z = 0.5 highlights essential differences in critical behavior along the Gaussian transition line.The Gaussian transition appears in several fields of quantum physics and statistical mechanics. The equivalence between surface-roughening transitions in classical two-dimensional (2D) models and quantum phase transitions in spin chains was introduced in Ref. 1, and their rich phase diagrams were investigated at length in Ref. 2. Characterized by continuously variable exponents, the Gaussian transition differs significantly both from regular phase transitions and from those of Kosterlitz-Thouless (KT) type. These differences complicate both analytical and numerical approaches to a complete and accurate description of rough surfaces and quantum spin chains.The S = 1 Heisenberg chain is one of the fundamental models in quantum magnetism. It formed the basis of Haldane's conjecture 3 for a finite gap in antiferromagnetic chains with integer spin, as opposed to the gapless spectrum of half-odd-integer cases. Numerically, quantum spin chains are important test cases for any computational technique, and Haldane's prediction has been verified by a range of methods with increasing accuracy. 4,5 Experimentally, while the "Haldane gap" has been found in the excitation spectra of many systems, 6 most known S = 1 chains, 9 are organic Ni materials with significant single-ion anisotropies. Analytical approaches to the Gaussian transition driven by this term are complicated by the lack of a suitable effective field theory, 10 and its broad nature makes all numerical techniques difficult to apply. Many authors have considered this transition, producing occasionally contradictory results. [11][12][13][14][15][16][17][18][19] In this Rapid Communication we resolve the problem of the Gaussian transition in the S = 1 chain with single-ion anisotropy. We exploit the fact that this transition is a gapless point between two gapped phases, whence the entropy exhibits a sharp peak. We introduce an improved density-matrix renormalization group (DMRG) approach with systematic error control, allowing high-precision calculations at system sizes up to L = 20 000, which automatically eliminate the endspin entropy. We determine the critical point with very high accuracy, and thereby deduce the critical behavior of several quantities at different...