“…[ 3 , 4 ] Among various TIs, bismuth antimony trichalcogenides (Bi,Sb) 2 Ch 3 ( Ch = S, Se, and Te) and their derivatives have emerged as the most promising material platform due to their large bulk gap of ≈0.3 eV, a simple TSS having a single Dirac cone with helical spin texture, and van der Waals (vdW) layered structure, which are favorable for suppressing the bulk contribution, enhancing charge‐to‐spin conversion, and realizing atomically clean interface for high spin transparency, respectively. [ 5 , 6 , 7 , 8 , 9 , 10 , 11 , 12 , 13 , 14 , 15 ] Various types of ferromagnet (FM) layers have been deposited on top of the (Bi,Sb) 2 Ch 3 ‐type TI layers for the SOT devices, demonstrating more efficient SOT operation compared to the HM/FM devices. [ 16 , 17 , 18 , 19 , 20 ] However, all‐vdW TI/FM heterostructure devices, in which strong charge‐to‐spin conversion and high interfacial spin transparency can be achieved simultaneously at room temperature, have rarely been studied, partly due to the lack of suitable vdW FMs.…”