A systematic comparative study of the electronic transport and ferromagnetic resonance of ultrathin trilayers (TLs) of SrRuO3/LaNiO3/ La0.7Sr0.3MnO3 on (001)-and (111)-oriented SrTiO3 (STO) substrates has been reported. An unusual upturn in resistivity ρ(T) at low-temperature (so called Kondo-like behaviour) accompanied by the negative magneto-resistance has been observed. For temperatures larger than the Kondo temperature (TK), ρ(T) is in good agreement with the Hamann's impurity resistivity model ρ(T >TK) ∝ (ln(T /TK)) −2 for spin S=1/2 and 3/2 for the TLs on (001)-STO and (111)-STO, respectively. At the temperatures T ≫ TK, electron-electron (ρ(T)∝ T 2) contribution dominates over those appearing due to the electron-phonon interaction (ρ(T)∝ T 5) and 2-Magnon scattering. Using the ferromagnetic resonance near the Curie temperature of La0.7Sr0.3MnO3, we evaluated the contribution of surface anisotropies (Ks) as well as in-plane volume anisotropies (Kν) : Ks ∼ −9.57 × 10 −4 J/m 2 (-6.68 ×10 −4 J/m 2) and Kν ∼ 4.04 × 10 5 J/m 3 (3.31×10 5 J/m 3) for the TLs on (001)-STO (TLs on (111)-STO). In addition, the Gilbert damping constant is determined which varies between 0.32 (0.23) and 0.16 (0.19) having spin mixing conductance, g ↑↓ = 5.2×10 19 m −2 (13.38×10 19 m −2) for TLs on (001)-STO ((111)-STO).