“…The complex electronic structure of uranium leads to a wide variety of unusual and diverse behavior in the uranium salts UX (X = C, N, P, S, As, Se, Sb, Te, Bi), and therefore the materials in this family have been the subject of many past investigations characterizing their magnetic and vibrational properties [1][2][3][4][5][6][7][8][9][10]. The phonon spectra in the UX systems have been comprehensively studied, however there has been renewed interest in more detailed calculations of their vibrational properties as certain members of the family, including UN and UC, are under active consideration for next generation nuclear fuels [11][12][13].…”