Isomer shifts have been determined in [111][112][113][114][115][116][117][118][119][120][121][122][123][124][125][126][127][128][129] Cd by high-resolution laser spectroscopy at CERN-ISOLDE. The corresponding mean square charge-radii changes, from the 1=2 þ and the 3=2 þ ground states to the 11=2 − isomers, have been found to follow a distinct parabolic dependence as a function of the atomic mass number. Since the isomers have been previously associated with simplicity due to the linear mass dependence of their quadrupole moments, the regularity of the isomer shifts suggests a higher order of symmetry affecting the ground states in addition. A comprehensive description assuming nuclear deformation is found to accurately reproduce the radii differences in conjunction with the known quadrupole moments. This intuitive interpretation is supported by covariant density functional theory. DOI: 10.1103/PhysRevLett.116.032501 Complexity is known to dominate the nuclear state, hence, sustaining the need for theoretical input to nearly every experimental work in order to disentangle the nuclear problem down to a set of basic concepts, e.g., shell structure, pairing, "magic" numbers, deformation, etc. However, in near-closed-shell nuclei, simple structures may occur as a result of the spherical symmetry breaking up. The cadmium isotopic chain studied here appears to provide one such instance of simplicity.Already [4,5] or states in the same nucleus [6]. Thus far, radial changes of such magnitude appear to be uncommon, the other prominent examples being the halo structures in light nuclei [7][8][9][10][11] and the onset of deformation at N ¼ 60 [12][13][14][15][16]. Cadmium and mercury are analogues in terms of their charge distributions since both incorporate an open shell with two protons less than a magic number, respectively, Z ¼ 50 and Z ¼ 82. Despite the similarities, the cadmium case presented here shows no abrupt changes of the nuclear size. Instead, one observes a small-to-moderate effect on the radii characterized by regularity which may be attributed to the unique-parity h 11=2 orbital.In this Letter, we report on the simplicity of high-precision isomer shifts derived from collinear laser spectroscopy on the neutron-rich cadmium isotopes towards the N ¼ 82 shell closure. A comprehensive model resting on some of the basic concepts in nuclear physics suggests an apparent link between the 11=2 − radii and quadrupole moments. The credibility of such an interpretation is examined quantitatively within a relativistic mean field calculation.The work was carried out with the collinear laser spectroscopy setup at the CERN-ISOLDE radioactivebeam facility. Of interest were the odd neutron-rich