2024
DOI: 10.1002/adma.202403873
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Spontaneous Supercrystal Formation During a Strain‐Engineered Metal–Insulator Transition

Oleg Yu. Gorobtsov,
Ludi Miao,
Ziming Shao
et al.

Abstract: Mott metal–insulator transitions possess electronic, magnetic, and structural degrees of freedom promising next‐generation energy‐efficient electronics. A previously unknown, hierarchically ordered, and anisotropic supercrystal state is reported and its intrinsic formation characterized in‐situ during a Mott transition in a Ca2RuO4 thin film. Machine learning‐assisted X‐ray nanodiffraction together with cryogenic electron microscopy reveal multi‐scale periodic domain formation at and below the film transition … Show more

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