SrTiO3–TiO2 Litchi-Like Hollow Nanospheres for Superior Photocatalytic Hydrogen Production

Yang, Yuhao; Zhang, Yixia; Wang, Tingting; Ma, Yongning; Xing, Shushu; Yan, Jiahao; Ran, Jie; Li, Xiaolong

doi:10.1007/s10562-023-04543-4

Cited by 4 publications

(1 citation statement)

References 55 publications

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“…Specifically, the flat-band potential for g-C 3 N 4 was approximately −1.6 eV, while for MoS 2 NTs, it was around −0.13 eV. Given that the conduction band potential of n-type semiconductors closely aligns with the flat-band potential, we approximated the flat-band potential as the conduction band potential for subsequent calculations . To approximate the band structure based on the bandgap diagrams and Mott–Schottky curves of MoS 2 NTs and g-C 3 N 4 , it can be calculated using the following formula: E CB = E VB - E g , where E CB is the valence band potential (eV); E VB is the conduction potential (eV); E g is the Band gap (eV).…”

Section: Resultsmentioning

confidence: 99%

Boosting the Photocatalytic Performance of g-C₃N₄ through MoS₂ Nanotubes with the Cavity Enhancement Effect

Li,

Zhang,

Wei

et al. 2024

Langmuir

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The development of catalysts with high photon utilization efficiency is crucial for enhancing the catalytic performance of photocatalysts. Graphitic carbon nitride (g-C3N4) is a prominent material in the field of photocatalysis. However, it still exhibits drawbacks such as low utilization of visible light and severe recombination of photogenerated carriers. To address these issues, this study employs MoS2 nanotubes (NTs) as cocatalysts and constructs MoS2 NTs/g-C3N4. The MoS2 NTs/g-C3N4 exhibits a significant cavity enhancement effect through multiple light reflections. This results in a broad spectral absorption range and high photon utilization efficiency, while also reducing the recombination of photogenerated carriers. The photocatalyst demonstrates outstanding performance in both photocatalytic hydrogen production and photodegradation of organic pollutants. Specifically, the hydrogen production rate is 1921 μmol·g–1·h–1, which is approximately 2.4 times that of g-C3N4. Furthermore, the photodegradation rate of Rhodamine B reaches 98.6% within 30 min, which is approximately three times higher than that of g-C3N4. Free radical capture experiments confirm that holes (h+) are the primary active species in photodegradation. A plausible photocatalytic mechanism for the catalyst is proposed. This study provides valuable insights into the development of heterojunction photocatalysts with high photon utilization efficiency.

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Section: Resultsmentioning

confidence: 99%

Boosting the Photocatalytic Performance of g-C₃N₄ through MoS₂ Nanotubes with the Cavity Enhancement Effect

Li,

Zhang,

Wei

et al. 2024

Langmuir

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CO2 photoconversion using photocatalyst of TiO2 thin films deposited by sputtering technique

Cruz,

Ceballos-Sanchez,

Rodríguez-Rocha

et al. 2024

J Mater Sci: Mater Electron

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Enhanced photocatalytic hydrogen production using TiO2 nanoflower photocatalysts loaded with Zn-Cu-In-Se quantum dots

Geng,

Yuan,

Wang

et al. 2024

Journal of Crystal Growth

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SrTiO3–TiO2 Litchi-Like Hollow Nanospheres for Superior Photocatalytic Hydrogen Production

Cited by 4 publications

References 55 publications

Boosting the Photocatalytic Performance of g-C₃N₄ through MoS₂ Nanotubes with the Cavity Enhancement Effect

Boosting the Photocatalytic Performance of g-C₃N₄ through MoS₂ Nanotubes with the Cavity Enhancement Effect

CO2 photoconversion using photocatalyst of TiO2 thin films deposited by sputtering technique

Enhanced photocatalytic hydrogen production using TiO2 nanoflower photocatalysts loaded with Zn-Cu-In-Se quantum dots

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SrTiO3–TiO2 Litchi-Like Hollow Nanospheres for Superior Photocatalytic Hydrogen Production

Cited by 4 publications

References 55 publications

Boosting the Photocatalytic Performance of g-C3N4 through MoS2 Nanotubes with the Cavity Enhancement Effect

Boosting the Photocatalytic Performance of g-C3N4 through MoS2 Nanotubes with the Cavity Enhancement Effect

CO2 photoconversion using photocatalyst of TiO2 thin films deposited by sputtering technique

Enhanced photocatalytic hydrogen production using TiO2 nanoflower photocatalysts loaded with Zn-Cu-In-Se quantum dots

Contact Info

Product

Resources

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Boosting the Photocatalytic Performance of g-C₃N₄ through MoS₂ Nanotubes with the Cavity Enhancement Effect

Boosting the Photocatalytic Performance of g-C₃N₄ through MoS₂ Nanotubes with the Cavity Enhancement Effect