“…This choice was guided by a number of previously reported investigations: first, dealing with the linear properties of such liquid-core PCFs and showing that the transmission spectral band and the zero-dispersion wavelength do not only depend on the microstructuring geometry of the fiber, but also on the linear refractive index of the filling liquid [29]; and second addressing their nonlinear properties, focusing on two main aspects: 1) The self-phase modulation process [2] has been exploited to measure the nonlinear refractive indices of liquids [30,31], and 2) The stimulated Raman scattering process has been extensively studied [32][33][34][35], leading to the development of efficient single-mode Raman converters with high spectral flexibility. These converters take advantage of both the special Raman properties of liquids (particularly their usual thin-line Raman spectra, with typical widths in the tens of GHz range, i.e., two to three orders of magnitude thinner than the 7-THz-FWHM Raman spectrum of silica) and the flexibility of the liquid-core fiber architecture in terms of transmission band positioning (see [32][33][34][35] for more details). Our point is that these two features can be also exploited to drastically reduce the SpRS noise in fibered sources of correlated photon pairs: by adequately choosing the microstructuring geometry of the hollow-core PCF, the linear refractive index of the liquid, and the pump wavelength, it becomes possible to generate the photon pairs outside the thin Raman lines of the liquid (which is not possible with the broad continua of the Raman spectra in glass materials).…”